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Chromium steel from chromite ore processing residue----A valuable construction material from a waste

Jay N. MEEGODA, Wiwat KAMOLPORNWIJIT

《环境科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 159-166 doi: 10.1007/s11783-011-0325-3

摘要： As species we humans generate excessive amounts of waste and hence for sustainability we should explore innovative ways to recover them. The primary objective of this study is to demonstrate an efficient and optimum way to recover chromium and iron from chromite ore processing residues (COPR) for the production of chrome steel and stainless steel. In Hudson County, New Jersey, there are more than two million tons of leftover COPR. Part of COPR was used as fill materials for construction sites, which spread the problem to a larger area. With high solubility along with their toxicity leached chromate from COPR is threatening the environment as well as human health. In this research, COPR was thermally treated to recover iron with chromium by applying techniques used in steel manufacturing. An extensive experimental program was performed using a Thermo-Gravimetric Analyzer (TGA) and bench scale tests to thermally treat the processed chromium contaminated soils with carbon and sand at varying temperatures and under reducing environment. The optimum chemical composition of COPR and additives to be used in the melts were evaluated based upon the thermodynamic properties of the mixture to ensure good phase separation, least amounts of iron and chromium oxides in the slag and minimum variability of final product (steel or iron with chromium). The impact of other oxides on the steel making process was evaluated to minimize the adverse impact on the process. The research demonstrated the feasibility of recovering a valuable construction material (chrome steel) from a waste (COPR).

关键词： chromite ore processing residue     chromium steel     reduction     thermal treatment     beneficial use    

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迈向21世纪的炼油技术

侯芙生

《中国工程科学》 1999年 第1卷 第3期   页码 22-30

摘要：

21世纪石油仍将是主要能源，炼油技术将进一步发展。降低汽车排放污染的清洁汽油生产技术，低硫低芳清洁柴油生产技术，加氢法润滑油基础油生产技术，加氢裂化和催化裂化重质油转化技术，渣油加工和能量综合利用技术，炼油厂现代化信息技术和过程控制技术等，将成为迈向21世纪有发展前途的炼油技术。

关键词： 炼油技术     清洁燃料     重油转化     渣油加工     过程控制    

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Emission factors of gaseous carbonaceous species from residential combustion of coal and crop residue

Qin WANG, Chunmei GENG, Sihua LU, Wentai CHEN, Min SHAO

《环境科学与工程前沿（英文）》 2013年 第7卷 第1期   页码 66-76 doi: 10.1007/s11783-012-0428-5

摘要： Experiments were performed to measure the emission factors ( s) of gaseous carbonaceous species, such as CO , CO, CH , and non-methane volatile organic compounds (NMVOCs), from the combustion of five types of coal of varying organic maturity and two types of biomass briquettes under residential burning conditions. Samples were collected in stainless steel canisters and 2,4-dinitrophenylhydrazine (DNPH) cartridges and were analyzed by GC–FID/MS and HPLC, respectively. The s from crop residue briquette burning were generally higher than those from coals, with the exception of CO . The dominant NMVOC species identified in coal smoke were carbonyls (41.7%), followed by C2 unsaturated hydrocarbons (29.1%) and aromatics (12.1%), while C2 unsaturated hydrocarbons were the dominant species (68.9%) emitted from the combustion of crop residue briquettes, followed by aromatics (14.4%). A comparison of burning normal crop residues in stoves and the open field indicated that briquettes emitted a larger proportion of ethene and acetylene. Both combustion efficiency and coal organic maturity had a significant impact on NMVOC s from burning coal: NMVOC emissions increased with increasing coal organic maturity but decreased as the combustion efficiency improved. Emissions from the combustion of crop residue briquettes from stoves occurred mainly during the smoldering process, with low combustion efficiency. Therefore, an improved stove design to allow higher combustion efficiency would be beneficial for reducing emissions of carbonaceous air pollutants.

关键词： residential combustion     coal     crop residue briquette     emission factors     gaseous carbonaceous species    

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Environmental, social, and economic assessment of energy utilization of crop residue in China

Yueling ZHANG, Junjie LI, Huan LIU, Guangling ZHAO, Yajun TIAN, Kechang XIE

《能源前沿（英文）》 2021年 第15卷 第2期   页码 308-319 doi: 10.1007/s11708-020-0696-x

摘要： This paper aims to discuss an environmental, social, and economic analysis of energy utilization of crop residues from life cycle perspectives in China. The methodologies employed to achieve this objective are environmental life cycle assessment (E-LCA), life cycle cost (LCC), and social life cycle assessment (S-LCA). Five scenarios are developed based on the conversion technologies and final bioenergy products. The system boundaries include crop residue collection, transportation, pre-treatment, and conversion process. The replaced amounts of energy are also taken into account in the E-LCA analysis. The functional unit is defined as 1 MJ of energy produced. Eight impact categories are considered besides climate change in E-LCA. The investment capital cost and salary cost are collected and compared in the life cycle of the scenarios. Three stakeholders and several subcategories are considered in the S-LCA analysis defined by UNEP/SETAS guidelines. The results show that the energy utilization of crop residue has carbon emission factors of 0.09–0.18 kg (CO eq per 1 MJ), and presents a net carbon emissions reduction of 0.03–0.15 kg (CO eq per 1 MJ) compared with the convectional electricity or petrol, but the other impacts should be paid attention to in the biomass energy scenarios. The energy utilization of crop residues can bring economic benefit to local communities and the society, but the working conditions of local workers need to be improved in future biomass energy development.

关键词： crop residue     life cycle assessment     life cycle cost     social life cycle assessment     energy production    

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Assessing the potential of crop residue recycling in China and technology options based on a bottom-up

Lili QU,Tianzhu ZHANG,Wei LU

《环境科学与工程前沿（英文）》 2014年 第8卷 第4期   页码 570-579 doi: 10.1007/s11783-013-0604-2

摘要： Crop residues are an important biomass, and are significant in the sustainable development of China. This paper uses the Grey-Markov modeling approach, the cost-benefit analysis method, and the constraint optimization method to establish the potential of crop residue recycling in China (CRRC) using a bottom-up analysis. Taking 2010 as the baseline year, the CRRC model is used to determine the quantity trends of crop residue resources, simulating the recycling potential and selecting key crop residue recycling technologies for operation between 2010 and 2030. The results illustrate that the total residue output from different crops will gradually increase to 1062 million tons in 2030. The proportion of crop residue for field burning is expected to decrease as a result of guidance and support from the government. Market mechanisms are also improving the development of the crop residue recycling industry. The economic benefit of crop residue recycling is expected to be worth 132 billion CNY in 2030 according to technology structure options. Key crop residue recycling technologies preferred such as liquefaction, amination, silo, co-firing straw power and composting will account for more than 85% of the total benefits.

关键词： China     crop residue     recycling potential     technology options    

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Porous silica synthesis out of coal fly ash with no residue generation and complete silicon separation

《环境科学与工程前沿（英文）》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1712-2

摘要：

● Both amorphous and crystalline silicon are completely separated from coal fly ash.

关键词： Coal fly ash     Alkali fusion     Micro-/meso-porous Si     Zeolite MCM-48     Crystalline transformation    

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Immobilized

Pei MA, Dan ZHANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 498-508 doi: 10.1007/s11783-012-0429-4

摘要： To investigate the potential use of ( ) residue for Cd adsorption, poly alcohol Na alginate (PVA) was applied to immobilize it. The parameters including contact time, pH, adsorbent dosages, and coexisting metal ions were studied. The suitable pH for immobilized was 4–7 wider than that for raw (pH 6–7). In the presence of Pb concentration varying from 0 to 30 mg·L , the Cd adsorption ratios declined by 6.71% and 47.45% for immobilized and raw , respectively. While, with the coexisting ion Cu concentration varied from 0 to 30 mg·L , the Cd adsorption ratios declined by 12.97% and 50.56% for immobilized and raw , respectively. The Cd adsorption isotherms in single–metal and dual-metal solutions were analyzed by using Langmuir, Freundlich, and Dubinin–Radushkevich models. The Cd adsorption capacities ( ) in single-metal solution were 6.448 mg·L and 2.832 mg·L for immobilized and raw , respectively. The of immobilized were 1.850 mg Cd·g in Cd + Pb solution and 3.961 mg Cd·g in Cd + Cu solution, respectively. The Cd adsorption processes subjected to both adsorbents follow pseudo-second-order model. Mechanism study showed the functional group of was –OH, –NH, –CO, and PVA played an important role in metal adsorbing. Mining wastewater treatment test showed that PVA–SA-immobilized was effective in mixed pollutant treatment even for wastewater containing metal ions in very low concentration.

关键词： immobilization     Lentinus edodes residue     competitive adsorption     isotherm    

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含铬废水常温合成铬铁矿的结晶行为及稳定性 Article

吕晋芳, 全英聪, 童雄, 彭勇军, 郑永兴

《工程（英文）》 2022年 第9卷 第2期   页码 67-76 doi: 10.1016/j.eng.2020.12.018

摘要：

铁氧体法不仅能净化含重金属废水，而且能从废水中回收有价金属。因此，铁氧体法被认为是一种处理含铬废水最具潜力的技术。然而，由于高的合成温度，该技术尚未在工业上得到广泛应用。本文对常温合成铬铁矿的可行性进行全面研究。考查了关键因素对出水水质、合成产物结晶行为和稳定性的影响。结果表明，经过常温铁氧体法处理后，废水中铬的去除率超过99.0%，上清液中铬的浓度达到污水排放标准。提高充气速率、搅拌速率和反应时间有利于稳定铬铁矿的形成。通过常温铁氧体法获得的颗粒结构致密，最大粒径可达52 μm。在合成过程中，铬逐渐地进入尖晶石晶体结构，合成铬铁矿的分子式为Fe3-xCrxO4，其中x约0.30。为阐明常温环境下铬铁矿的合成机理，提出了微观反应路径。本研究为铁氧体法在含铬废水净化和综合利用方面的工业应用奠定了基础。

关键词： 含铬废水     铬铁矿合成     常温     结晶行为     稳定性    

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Utilization of nano/micro-size iron recovered from the fine fraction of automobile shredder residue for

Jiwan SINGH, Yoon-Young CHANG, Jae-Kyu YANG, Seon-Hong KANG, Janardhan Reddy KODURU

《环境科学与工程前沿（英文）》 2016年 第10卷 第4期 doi: 10.1007/s11783-016-0848-8

摘要： Phenol removal by n/m Fe in the presence of H O was highly effective. Increasing the amounts of n/m Fe and H O ?increased the phenol removal rate. Phenol removal was decreased with an increase in the concentration of phenol. The natural pH (6.9) of the solution was highly effective for phenol removal. The pseudo-first-order kinetics was best fitted for the degradation of phenol. The study investigates the magnetic separation of Fe from automobile shredder residue (ASR) (<0.25 mm) and its application for phenol degradation in water. The magnetically separated Fe was subjected to an ultrasonically assisted acid treatment, and the degradation of phenol in an aqueous solution using nano/micro-size Fe (n/m Fe) was investigated in an effort to evaluate the possibility of utilizing n/m Fe to remove phenol from wastewater. The prepared n/m Fe was analyzed by scanning electron microscopy (SEM) and Fourier transform infrared spectroscopy (FTIR). The effects of the dosages of n/mFe, pH, concentration of phenol and amount of H O on phenol removal were evaluated. The results confirm that the phenol degradation rate was improved with an increase in the dosages of n/mFe and H O ; however, the rate is reduced when the phenol concentration is higher. The degradation of phenol by n/mFe followed the pseudo-first-order kinetics. The value of the reaction rate constant ( was increased as the amounts of n/m Fe and H O increased. Conversely, the value of was reduced when the concentration of phenol was increased. The probable mechanism behind the degradation of phenol by n/m Fe is the oxidation of phenol through hydroxyl radicals which are produced during the reaction between H O and n/m Fe.

关键词： Automobile shredder residue (ASR)     Fe     Phenol     Scanning electron microscopy (SEM) and Fourier transform infrared spectroscopy (FTIR)     Mechanism    

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Green process to recover magnesium chloride from residue solution of potassium chloride production plant

WANG Lin, HE Yunliang, WANG Yanfei, BAO Ying, WANG Jingkang

《化学科学与工程前沿（英文）》 2008年 第2卷 第4期   页码 385-389 doi: 10.1007/s11705-008-0079-z

摘要： The green process to recover magnesium chloride from the residue solution of a potassium chloride production plant, which comes from the leach solution of a potash mine in Laos, is designed and optimized. The residue solution contains magnesium chloride above 25 wt-%, potassium chloride and sodium chloride together below 5 wt-% and a few other ions such as Br, SO and Ca. The recovery process contains two steps: the previous impurity removal operation and the two-stage evaporation-cooling crystallization procedure to produce magnesium chloride. The crystallized impurity carnallite obtained from the first step is recycled to the potassium chloride plant to recover the potassium salt. The developed process is a zero discharge one and thus fulfills the requirements for green chemical industrial production. The produced magnesium chloride is up to industrial criteria.

关键词： industrial production     chemical industrial     produced magnesium     chloride production     impurity carnallite    

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Review on flexible perovskite photodetector: processing and applications

《机械工程前沿（英文）》 2023年 第18卷 第2期 doi: 10.1007/s11465-023-0749-z

摘要： Next-generation optoelectronics should possess lightweight and flexible characteristics, thus conforming to various types of surfaces or human skins for portable and wearable applications. Flexible photodetectors as fundamental devices have been receiving increasing attention owing to their potential applications in artificial intelligence, aerospace industry, and wise information technology of 120, among which perovskite is a promising candidate as the light-harvesting material for its outstanding optical and electrical properties, remarkable mechanical flexibility, low-cost and low-temperature processing methods. To date, most of the reports have demonstrated the fabrication methods of the perovskite materials, materials engineering, applications in solar cells, light-emitting diodes, lasers, and photodetectors, strategies for device performance enhancement, few can be seen with a focus on the processing strategies of perovskite-based flexible photodetectors, which we will give a comprehensive summary, herein. To begin with, a brief introduction to the fabrication methods of perovskite (solution and vapor-based methods), device configurations (photovoltaic, photoconductor, and phototransistor), and performance parameters of the perovskite-based photodetectors are first arranged. Emphatically, processing strategies for photodetectors are presented following, including flexible substrates (i.e., polymer, carbon cloth, fiber, paper, etc.), soft electrodes (i.e., metal-based conductive networks, carbon-based conductive materials, and two-dimensional (2D) conductive materials, etc.), conformal encapsulation (single-layer and multilayer stacked encapsulation), low-dimensional perovskites (0D, 1D, and 2D nanostructures), and elaborate device structures. Typical applications of perovskite-based flexible photodetectors such as optical communication, image sensing, and health monitoring are further exhibited to learn the flexible photodetectors on a deeper level. Challenges and future research directions of perovskite-based flexible photodetectors are proposed in the end. The purpose of this review is not only to shed light on the basic design principle of flexible photodetectors, but also to serve as the roadmap for further developments of flexible photodetectors and exploring their applications in the fields of industrial manufacturing, human life, and health care.

关键词： photodetector     perovskite     flexible     processing     application    

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The effect of pH, solid content, water chemistry and ore mineralogy on the galvanic interactions between

Asghar Azizi, Seid Ziaoddin Shafaei, Mohammad Noaparast, Mohammad Karamoozian

《化学科学与工程前沿（英文）》 2013年 第7卷 第4期   页码 464-471 doi: 10.1007/s11705-013-1356-z

摘要： The role of pH, solid content, water chemistry and ore mineralogy on the galvanic interactions between chalcopyrite and pyrite and low alloy steel balls were investigated in the grinding of Sarcheshmeh porphyry copper sulfide ore. All these factors strongly affect the galvanic current between the minerals and the steel during the grinding process. The galvanic current density decreased as the solution pH and percent solids increased. In addition, changing the water in the ball mill from tap to distilled water reduced the galvanic current between the minerals and the balls. Potentiodynamic polarization curves showed that pyrite and chalcopyrite demonstrated typical active-passive-transpassive anodic behavior in the grinding of copper ore. However, the nature of their transitions from the active to the passive state differed. This behavior was not seen in the grinding of pure minerals. In addition, an EDTA extraction technique was employed to quantify the amount of oxidized iron in the mill discharge. The amount of extractable iron was influenced by the same experimental factors and in the same way as the galvanic current.

关键词： steel ball     galvanic interaction     pyrite     chalcopyrite     polarization curves    

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Oxidative leaching kinetics of molybdenum-uranium ore in H

T. A. Lasheen, M. E. El-Ahmady, H. B. Hassib, A. S. Helal

《化学科学与工程前沿（英文）》 2013年 第7卷 第1期   页码 95-102 doi: 10.1007/s11705-013-1317-6

摘要： The processing of molybdenum-uranium ore in a sulfuric acid solution using hydrogen peroxide as an oxidant has been investigated. The leaching temperature, hydrogen peroxide concentration, sulfuric acid concentration, leaching time, particle size, liquid-to-solid ratio and agitation speed all have significant effects on the process. The optimum process operating parameters were: temperature: 95°C; H O concentration: 0.5 M; sulfuric acid concentration: 2.5 M; time: 2 h; particle size: 74 μm, liquid-to-solid ratio: 14 ∶ 1 and agitation speed: 600 rpm. Under these experimental conditions, the extraction efficiency of molybdenum was about 98.4%, and the uranium extraction efficiency was about 98.7%. The leaching kinetics of molybdenum showed that the reaction rate of the leaching process is controlled by the chemical reaction at the particle surface. The leaching process follows the kinetic model 1 ? (1? ) = with an apparent activation energy of 40.40 kJ/mole. The temperature, concentrations of H O and H SO and the mesh size are the main factors that influence the leaching rate. The reaction order in H SO was 1.0012 and in H O it was 1.2544.

关键词： leaching of molybdenum     leaching of uranium     kinetics    

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中国的小岩体岩浆矿床

汤中立

《中国工程科学》 2002年 第4卷 第6期   页码 9-12

摘要：

我国没有发现与巨型层状岩体有关的岩浆矿床，但是在许多小岩体中，却发现了超大型和大型的岩浆矿床；提出了小岩体岩浆矿床是今后一个重要的研究和勘查方向。

关键词： 小岩体     岩浆矿床     勘查    

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Assessment of popular techniques for co-processing municipal solid waste in Chinese cement kilns

《环境科学与工程前沿（英文）》 2022年 第16卷 第4期 doi: 10.1007/s11783-021-1485-4

摘要：

• Municipal solid waste (MSW) was fermented, screened, gasified, then co-processed.

关键词： Cement kiln     Co-processing     Environmental risk assessment     By-pass system    

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标题 作者 时间 类型 操作

Chromium steel from chromite ore processing residue----A valuable construction material from a waste

Jay N. MEEGODA, Wiwat KAMOLPORNWIJIT

期刊论文

迈向21世纪的炼油技术

侯芙生

期刊论文

Emission factors of gaseous carbonaceous species from residential combustion of coal and crop residue

Qin WANG, Chunmei GENG, Sihua LU, Wentai CHEN, Min SHAO

期刊论文

Environmental, social, and economic assessment of energy utilization of crop residue in China

Yueling ZHANG, Junjie LI, Huan LIU, Guangling ZHAO, Yajun TIAN, Kechang XIE

期刊论文

Assessing the potential of crop residue recycling in China and technology options based on a bottom-up

Lili QU,Tianzhu ZHANG,Wei LU

期刊论文

Porous silica synthesis out of coal fly ash with no residue generation and complete silicon separation

期刊论文

Immobilized

Pei MA, Dan ZHANG

期刊论文

含铬废水常温合成铬铁矿的结晶行为及稳定性

吕晋芳, 全英聪, 童雄, 彭勇军, 郑永兴

期刊论文

Utilization of nano/micro-size iron recovered from the fine fraction of automobile shredder residue for

Jiwan SINGH, Yoon-Young CHANG, Jae-Kyu YANG, Seon-Hong KANG, Janardhan Reddy KODURU

期刊论文

Green process to recover magnesium chloride from residue solution of potassium chloride production plant

WANG Lin, HE Yunliang, WANG Yanfei, BAO Ying, WANG Jingkang

期刊论文

Review on flexible perovskite photodetector: processing and applications

期刊论文

The effect of pH, solid content, water chemistry and ore mineralogy on the galvanic interactions between

Asghar Azizi, Seid Ziaoddin Shafaei, Mohammad Noaparast, Mohammad Karamoozian

期刊论文

Oxidative leaching kinetics of molybdenum-uranium ore in H

T. A. Lasheen, M. E. El-Ahmady, H. B. Hassib, A. S. Helal

期刊论文

中国的小岩体岩浆矿床

汤中立

期刊论文

Assessment of popular techniques for co-processing municipal solid waste in Chinese cement kilns

期刊论文